I keep failing ungracefully at a seemingly simple task of determing a function to describe the coherence between two measured variables (a, b) and and a resulting value. Here's a complete round of example measurements and their respective result:

x: -0.08 y: -0.28 result: 1.850
x: -0.16 y: -0.25 result: 2.129
x: -0.23 y: -0.19 result: 2.446
x: -0.26 y: -0.11 result: 2.744
x: -0.27 y: -0.03 result: 3.047
x: -0.25 y: +0.06 result: 3.363
x: -0.20 y: +0.13 result: 3.730
x: -0.14 y: +0.20 result: 4.121
x: -0.05 y: +0.22 result: 4.498
x: +0.03 y: +0.22 result: 4.844
x: +0.11 y: +0.19 result: 5.240
x: +0.19 y: +0.14 result: 5.652
x: +0.22 y: +0.08 result: 5.956
x: +0.26 y: -0.01 result: 6.330
x: +0.25 y: -0.10 result: 6.645
x: +0.21 y: -0.18 result: 6.996
x: +0.18 y: -0.24 result: 7.229
x: +0.09 y: -0.29 result: 7.553
x: +0.00 y: -0.29 result: 7.844
x: -0.07 y: -0.28 result: 1.829

I've figured so far that $result = (something + 0.5) times pi $, but I can't figure out the $something$ part. x seems to move between -0.27 and +0.27, while y between -0.30 and 0.22. I've tried to visualize their behaviour in circles, for hopefully it brings help rather than further confusion:

Visualization

I seem to have forgotten how to go about solving such a task and been fiddling with Wolfram Alpha for some time now, but can't seem to get behind the concept. Please help!

To sum it all up, the question is: find a function to calculate result from x and y.

Relating $x$ and $y$

You're right that $x$ and $y$ are related by circles. In fact, by plotting $y$ against $x$, we have the following graph.

This looks pretty close to a circle. The radius of a circle is given by
$$
r = sqrtx^2 + y^2,
$$
so by taking the average of each $sqrtx^2 + y^2$ for your data we find that the radius is approximately $r approx 0.2653$ (to $4$ significant figures). We also find that the average of the $x$ values is $barx = -0.0085$, and the average of the $y$ values is $bary = -0.0505$. These give an estimate for the center of the circle.

The next graph shows the circle of radius $r = 0.2653$ and midpoint $(-0.0085, -0.0505)$ (orange) compared to the plot of your data (blue).

It seems to fit fairly well.

Introducing $theta$

Assuming that this is 'good enough', we can parametrise your $(x, y)$ coordinates by replacing the $2$-tuple $(x, y)$ with $theta$, namely the angle that the point $(x, y)$ makes with the positive $x$-axis. The formula for $theta$ has a few different formulations depending on what range you want $theta$ in, but by playing around with the trigonometric identities you can determine which one you want. The formula that I used is
$$
theta = begincases
arctan(y/x),& textif $x > 0$,\
pi + arctan(y/x),& textif $x < 0$,\
mathrmsgn(y)pi/2,& textif $x = 0$.\
endcases
$$
Note that $mathrmsgn(y)$ is the function that returns the sign of $y$, so
$$
mathrmsgn(y) = begincases
+1,& textif $y > 0$,\
-1,& textif $y < 0$,\
0,& textif $y = 0$.\
endcases
$$
Plotting $theta$ against result, we have the following graph.

Performing simple linear regression on this gives the formula
$$
textresult = 6.2865 - theta.tag$ast$
$$
The values have been rounded to $4$ decimal places. Note that
$$
6.2865 approx 6.283185307 approx 2pi.
$$
The following graph shows how close the fit is.

The blue dots are the original data, and the orange dots are defined by the line $(ast)$

Defining the function

Now that we know the relationship, we can write up an estimate for your function. We will suppose that the constant in $(ast)$ is indeed $2pi$. If
$$
textresult = 2pi - theta
$$
and
$$
theta = begincases
arctan(y/x),& textif $x > 0$,\
pi + arctan(y/x),& textif $x < 0$,\
mathrmsgn(y)pi/2,& textif $x = 0$,\
endcases
$$
then it is easy to see that
$$
textresult = begincases
2pi - arctan(y/x),& textif $x > 0$,\
pi - arctan(y/x),& textif $x < 0$,\
2pi - mathrmsgn(y)pi/2,& textif $x = 0$.\
endcases
$$
The following tables shows how close the values are using this function. The real results are in the 'result' column, and the values using the function are in the 'forecast' column.
$$
beginarrayc
x & y & textresult & theta & textforecast\hline
-0.08 & -0.28 & colorred1.849 & 4.434 & colorgreen1.85 \
-0.16 & -0.25 & colorred2.14 & 4.143 & colorgreen2.129 \
-0.23 & -0.19 & colorred2.451 & 3.832 & colorgreen2.446 \
-0.26 & -0.11 & colorred2.741 & 3.542 & colorgreen2.744 \
-0.27 & -0.03 & colorred3.031 & 3.252 & colorgreen3.047 \
-0.25 & 0.06 & colorred3.377 & 2.906 & colorgreen3.363 \
-0.2 & 0.13 & colorred3.718 & 2.565 & colorgreen3.73 \
-0.14 & 0.2 & colorred4.102 & 2.182 & colorgreen4.121 \
-0.05 & 0.22 & colorred4.489 & 1.794 & colorgreen4.498 \
0.03 & 0.22 & colorred4.848 & 1.435 & colorgreen4.844 \
0.11 & 0.19 & colorred5.237 & 1.046 & colorgreen5.24 \
0.19 & 0.14 & colorred5.648 & 0.635 & colorgreen5.652 \
0.22 & 0.08 & colorred5.934 & 0.349 & colorgreen5.956 \
0.26 & -0.01 & colorred6.322 & -0.038 & colorgreen6.33 \
0.25 & -0.1 & colorred6.664 & -0.381 & colorgreen6.645 \
0.21 & -0.18 & colorred6.992 & -0.709 & colorgreen6.996 \
0.18 & -0.24 & colorred7.21 & -0.927 & colorgreen7.229 \
0.09 & -0.29 & colorred7.553 & -1.27 & colorgreen7.553 \
0 & -0.29 & colorred7.854 & -1.571 & colorgreen7.844 \
-0.07 & -0.28 & colorred1.816 & 4.467 & colorgreen1.829 \
endarray
$$
All values are rounded to $3$ decimal places.